Embrujaste is the past tense of the verb embrujar, meaning "to bewitch" or "to cast a spell on". It's a dramatic and poetic word you won't find in many songs.
In this track, the singer is so unable to get over his ex that he asks, "¿Será que embrujaste a este viejo triste?" (Could it be that you bewitched this sad old man?). He uses this word to express the almost supernatural hold this person still has on him, making it a powerful and memorable way to describe heartbreak.
VPPMHDSPPM by Los Gemelos De Sinaloa is a furious, alcohol-soaked vent session about an ex who won't get out of his head. The crazy title is actually an acronym for the song's most profane, explosive hook: "Vales pura pinche mierda, hija de su pinche perra puta madre" (You're worth absolutely nothing, you daughter of a bitch). He is stuck in heartbreak, complaining that even hanging out with three other girls ("Me la paso con tres morras") does nothing to erase her memory. Her kisses left a permanent mark, and he is spiraling so bad he wonders if she put a curse on him: "¿Será que embrujaste a este viejo triste?" (Did you put a spell on this sad old man?).
To cope, he hits the bottle hard, admitting, "Por tu culpa ando pisteando" (Because of you, I'm out drinking). In Mexican Spanish, pisteando comes from pistear, which specifically means drinking alcohol or partying hard. It is a messy mix of wounded ego and total despair. He knows he has too much self-worth to be chasing her all over the place ("Si supieras lo que valgo para andar buscándote por todos lados"), but he simply cannot stop himself.